Electroluminescence Generation in PbS Quantum Dot Light-Emitting Field-Effect Transistors with Solid-State Gating

Artem G. Shulga, Simon Kahmann, Dmitry N. Dirin, Arko Graf, Jana Zaumseil, Maksym V. Kovalenko, Maria A. Loi*

*Corresponding author for this work

Research output: Contribution to journalArticleAcademicpeer-review

47 Citations (Scopus)
337 Downloads (Pure)

Abstract

The application of light-emitting field-effect transistors (LEFET) is an elegant way of combining electrical switching and light emission in a single device architecture instead of two. This allows for a higher degree of miniaturization and integration in future optoelectronic applications. Here, we report on a LEFET based on lead sulfide quantum dots processed from solution. Our device shows state-of-the-art electronic behavior and emits near infrared photons with a quantum yield exceeding 1% when cooled. We furthermore show how LEFETs can be used to simultaneously characterize the optical and electrical material properties on the same device and use this benefit dot film. to investigate the charge transport through the quantum dot film.

Original languageEnglish
Pages (from-to)12805-12813
Number of pages9
JournalAcs Nano
Volume12
Issue number12
DOIs
Publication statusPublished - Dec-2018

Keywords

  • quantum dots
  • field-effect transistors
  • light emission
  • low temperature
  • traps
  • TEMPERATURE-DEPENDENT BEHAVIOR
  • SOLAR-CELLS
  • CHARGE-TRANSPORT
  • HIGH-MOBILITY
  • TRAP STATES
  • LOW-VOLTAGE
  • AMBIPOLAR
  • DENSITY
  • BRIGHT
  • FILMS

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