Exciton superradiance in molecular crystal slabs

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Abstract

We investigate the spontaneous emission rate γ of dipolar excitons in molecular crystal slabs of variable thickness, L, ranging from monolayers to bulk crystals. We find a smooth transition between superradiant excitons (γ ∝ L) at thickness small compared to an optical wavelength (λ) and radiatively stable polaritons for thick crystals (γ ∝ 1/L). The maximum cooperativity volume of the molecules in the slab is found to be of the order λ^3.
Original languageEnglish
Pages (from-to)101-104
Number of pages4
JournalJournal of Luminescence
Volume53
Issue number1-6
DOIs
Publication statusPublished - Jul-1992
Event8TH INTERNATIONAL CONF ON DYNAMICAL PROCESSES IN EXCITED STATES OF SOLIDS ( DPC 91 ) - , Netherlands
Duration: 27-Aug-199131-Aug-1991

Keywords

  • DEPENDENT RADIATIVE DECAY

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