Abstract
The fires around Moscow in July and August 2010 emitted a large amount
of pollutants to the atmosphere. Here we estimate the carbon monoxide
(CO) source strength of the Moscow fires in July and August by using the
TM5-4DVAR system in combination with CO column observations of the
Infrared Atmospheric Sounding Interferometer (IASI). It is shown that
the IASI observations provide a strong constraint on the total emissions
needed in the model. Irrespective of the prior emissions used, the
optimised CO fire emission estimates from mid-July to mid-August 2010
amount to approximately 24 Tg CO. This estimate depends only weakly
(<15%) on the assumed diurnal variations and injection height of the
emissions. However, the estimated emissions might depend on unaccounted
model uncertainties such as vertical transport. Our emission estimate of
22-27 Tg CO during roughly one month of intense burning is less than
suggested by another recent study, but substantially larger than
predicted by the bottom-up inventories. This latter discrepancy suggests
that bottom-up emission estimates for extreme peat burning events
require improvements.
Original language | English |
---|---|
Pages (from-to) | 4737-4747 |
Journal | Atmospheric Chemistry and Physics Discussions |
Volume | 13 |
Issue number | 9 |
DOIs | |
Publication status | Published - 1-May-2013 |