Close collisions in the two-dimensional Raman response of liquid carbon disulfide

TLC Jansen*, K Duppen, Jaap Snijders

*Bijbehorende auteur voor dit werk

OnderzoeksoutputAcademicpeer review

33 Citaten (Scopus)

Samenvatting

The fifth-order 2D Raman response of a liquid is calculated taking all possible interaction induced effects into account. Next to dipole-induced dipole interactions, close collision effects due to induced multipoles and electron overlap are found to give a significant contribution to the response of liquid carbon disulfide. A correct prediction of the spectrum is impossible, when these effects are not properly taken into account. The calculated response is found to be in good agreement with some of the most recent experiments.

Originele taal-2English
Artikelnummer134206
Pagina's (van-tot)art - 134206
Aantal pagina's5
TijdschriftPhysical Review. B: Condensed Matter and Materials Physics
Volume67
Nummer van het tijdschrift13
DOI's
StatusPublished - 1-apr-2003

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